I recently realized that the PLL is only using about 20% of the available actuation range of the AUX PZT. The +/-10 V control signal from the LB1005 is being directly inputted into the fast AUX PZT channel, which has an input range of +/-50 V.

I recommend to install a PZT driver (amplifier) between the controller and laser to use the full available actuator range. For cavity scans, this will increase the available sweep range from +/-50 MHz to +/-250MHz. This has a unique advantage even if slow temperature feedback is also implemented. To sample faster than the timescale of most of the angular noise,  scans generally need to be made with a total sweep time <1 sec. This is faster than the PLL offset can be offloaded via the slow temperature control, so the only way to scan more than 100 MHz in one measurement is with a larger dynamic range.