As Jenne mentioned, we took OLTF transfer functions, and determined that we had more than enough phase margin to switch on the LSC boosts in FM4. This improved the error signal noise spectra quite a lot, and noticeably reduced the TRX/TRY fluctuations, and actuation output.
Here's the CARM OLTF (FM4 boost on in red, boost off in black)

Here's what happened to the CARM and DARM spectra when we turned on the boosts. (ALS only in black, initial IR signal transitions in mid-color, boosted IR signals in bright color)
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